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ABSTRACT Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second‐order nonlinear processes, like second harmonic generation (SHG), typically require non‐centrosymmetric crystals to be realized. Here, we experimentally demonstrate enhanced SHG response by using a gold nanocavity array forming a plasmonic metasurface absorber where titanium dioxide (TiO₂), a centrosymmetric dielectric material, with subwavelength thickness, is deposited in the realized nanogaps. While such a dielectric material has an extremely low second‐order nonlinear susceptibility, we observe 10⁵‐fold boosting in the nonlinear SHG process mainly due to the surface nonlinear susceptibility of the gold metal, aided by the significant electric field enhancement that occurs in the nanogaps due to the formed nanocavity resonance. The experimental results obtained are theoretically explained with extensive and rigorous nonlinear simulations that consider all the bulk and surface linear and nonlinear material properties. The presented robust harmonic generation from an ultrathin plasmonic metasurface can be used in nonlinear and quantum integrated photonic applications. 

Abstract Efficient and compact single photon emission platforms operating at room temperature with ultrafast speed and high brightness will be fundamental components of the emerging quantum communications and computing fields. However, so far, it is very challenging to design practical deterministic single photon emitters based on nanoscale solid‐state materials that meet the fast emission rate and strong brightness demands. Here, a solution is provided to this longstanding problem by using metallic nanocavities integrated with hexagonal boron nitride (hBN) flakes with defects acting as nanoscale single photon emitters (SPEs) at room temperature. The presented hybrid nanophotonic structure creates a rapid speedup and large enhancement in single photon emission at room temperature. Hence, the nonclassical light emission performance is substantially improved compared to plain hBN flakes and hBN on gold‐layered structures without nanocavity. Extensive theoretical calculations are also performed to accurately model the new hybrid nanophotonic system and prove that the incorporation of plasmonic nanocavity is key to efficient SPE performance. The proposed quantum nanocavity single photon source is expected to be an element of paramount importance to the envisioned room‐temperature integrated quantum photonic networks. 

We experimentally demonstrate and theoretically verify a spectrally controllable, extremely large, broadband chiroptical response from three-dimensional all-dielectric broken L-shape nano-boomenrang metamaterial platforms. This innovative design holds great potential for seamless integration into on-chip photonic devices. 

Abstract Nanostructures represent a frontier where meticulous attention to the control and assessment of structural dimensions becomes a linchpin for their seamless integration into diverse technological applications. However, determining the critical dimensions and optical properties of nanostructures with precision still remains a challenging task. In this study, by using an integrative and comprehensive methodical series of studies, the evolution of the depolarization factors in the anisotropic Bruggeman effective medium approximation (AB‐EMA) is investigated. It is found that these anisotropic factors are extremely sensitive to the changes in critical dimensions of the nanostructure platforms. In order to perform a systematic characterization of these parameters, spatially coherent, highly‐ordered slanted nanocolumns are fabricated from zirconia, silicon, titanium, and permalloy on silicon substrates with varying column lengths using glancing angle deposition (GLAD). In tandem, broad‐spectral range Mueller matrix spectroscopic ellipsometry data, spanning from the near‐infrared to the vacuum UV (0.72–6.5 eV), is analyzed with a best‐match model approach based on the anisotropic Bruggeman effective medium theory. The anisotropic optical properties, including complex dielectric function, birefringence, and dichroism, are thereby extracted. Most notably, the research unveils a generalized, material‐independent inverse relationship between depolarization factors and column length. It is envisioned that the presented scaling rules will permit accurate prediction of optical properties of nanocolumnar thin films improving their integration and optimization for optoelectronic and photonic device applications. As an outlook, the highly porous nature and extreme birefringence properties of the fabricated columnar metamaterial platforms are further explored in the detection of nanoparticles from the cross‐polarized integrated spectral color variations. 

Abstract The inherently weak chiroptical responses of natural materials limit their usage for controlling and enhancing chiral light-matter interactions. Recently, several nanostructures with subwavelength scale dimensions were demonstrated, mainly due to the advent of nanofabrication technologies, as a potential alternative to efficiently enhance chirality. However, the intrinsic lossy nature of metals and the inherent narrowband response of dielectric planar thin films or metasurface structures pose severe limitations toward the practical realization of broadband and tailorable chiral systems. Here, we tackle these problems by designing all-dielectric silicon-based L-shaped optical metamaterials based on tilted nanopillars that exhibit broadband and enhanced chiroptical response in transmission operation. We use an emerging bottom-up fabrication approach, named glancing angle deposition, to assemble these dielectric metamaterials on a wafer scale. The reported strong chirality and optical anisotropic properties are controllable in terms of both amplitude and operating frequency by simply varying the shape and dimensions of the nanopillars. The presented nanostructures can be used in a plethora of emerging nanophotonic applications, such as chiral sensors, polarization filters, and spin-locked nanowaveguides. 

Graphene can support surface plasmons with higher confinement, lower propagation loss, and substantially more tunable response compared to usual metal-based plasmonic structures. Interestingly, plasmons in graphene can strongly couple with nanostructures and gratings placed in its vicinity to form new hybrid systems that can provide a platform to investigate more complicated plasmonic phenomena. In this Perspective, an analysis on the excitation of highly confined graphene plasmons and their strong coupling with metallic or dielectric gratings is performed. We emphasize the flexibility in the efficient control of light–matter interaction by these new hybrid systems, benefiting from the interplay between graphene plasmons and other external resonant modes. The hybrid graphene-plasmon grating systems offer unique tunable plasmonic resonances with enhanced field distributions. They exhibit a novel route to realize practical emerging applications, including nonreciprocal devices, plasmonic switches, perfect absorbers, nonlinear structures, photodetectors, and optical sensors.